Caulfield · Clinical chemistry 2008 · analytical validation study · n=?

Direct determination of lipoprotein particle sizes and concentrations by ion mobility analysis.

Cited 233 times in the scientific literature.

Level 5 - mechanism / opinion, no new human data

Laboratory analytical method validation using serum samples

PubMed 18515257 · doi:10.1373/clinchem.2007.100586 · record verified 2026-08-30

What was done

The authors developed and validated a gas-phase differential electrophoretic macromolecular mobility-based method (ion mobility, or IM) to directly measure the size and concentration of lipoprotein particles across subfractions from small, dense HDL to large VLDL (particle diameter range 17.2-540.0 A). Serum samples underwent an ultracentrifugation step to remove albumin before a 2-minute IM scan, and particle counts across predetermined size ranges were correlated with standard cholesterol and apolipoprotein measurements.

What was found

Intra- and interassay coefficients of variation for LDL particle size were <1.0%, and for LDL and HDL particle subfraction measurements were <20%. Ion mobility-measured non-HDL correlated strongly with apolipoprotein B (r = 0.92).

Why it matters

Ion mobility provides a direct physical measurement of lipoprotein particle sizes and subclass concentrations across a broad size spectrum. This offers a standardized method for lipid profiling that can be evaluated in clinical cardiovascular studies.

Limits

The abstract does not report the number or characteristics of human serum samples tested. Clinical utility, hard cardiovascular outcomes, and comparative performance against other subfraction assays were not evaluated.

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